000 02435nam a22004695i 4500
001 978-4-431-54043-4
003 DE-He213
005 20140220083333.0
007 cr nn 008mamaa
008 111122s2012 ja | s |||| 0|eng d
020 _a9784431540434
_9978-4-431-54043-4
024 7 _a10.1007/978-4-431-54043-4
_2doi
050 4 _aQD241-441
072 7 _aPSB
_2bicssc
072 7 _aSCI013040
_2bisacsh
072 7 _aSCI007000
_2bisacsh
082 0 4 _a547
_223
100 1 _aInuki, Shinsuke.
_eauthor.
245 1 0 _aTotal Synthesis of Bioactive Natural Products by Palladium-Catalyzed Domino Cyclization of Allenes and Related Compounds
_h[electronic resource] /
_cby Shinsuke Inuki.
264 1 _aTokyo :
_bSpringer Tokyo,
_c2012.
300 _aXVI, 106 p.
_bonline resource.
336 _atext
_btxt
_2rdacontent
337 _acomputer
_bc
_2rdamedia
338 _aonline resource
_bcr
_2rdacarrier
347 _atext file
_bPDF
_2rda
490 1 _aSpringer Theses
505 0 _aChapter 1. Total Synthesis of Pachastrissamine (Jaspine B) -- Chapter 2. Total Synthesis of Lysergic Acid, Lysergol, and Isolysergol -- Chapter 3. Conclusions.
520 _aThe author has developed novel methodologies for highly efficient construction of functionalized heterocycles by palladium-catalyzed domino/cascade cyclization of allenes and related compounds containing appropriate nucleophilic group(s). Based on these methodologies, enantioselective total syntheses of bioactive natural products, pachastrissamine (26% overall yield in seven steps), lysergic acid (4.0% overall yield in fifteen steps), lysergol (3.6% overall yield in fifteen steps) and isolysergol (8.2% overall yield in eleven steps) have been achieved. These are more facile synthetic route than those previously reported. These findings would contribute to the development of efficient synthetic methods for biologically active compounds containing a complex structure.
650 0 _aChemistry.
650 0 _aBioorganic chemistry.
650 0 _aCatalysis.
650 1 4 _aChemistry.
650 2 4 _aBioorganic Chemistry.
650 2 4 _aCatalysis.
710 2 _aSpringerLink (Online service)
773 0 _tSpringer eBooks
776 0 8 _iPrinted edition:
_z9784431540427
830 0 _aSpringer Theses
856 4 0 _uhttp://dx.doi.org/10.1007/978-4-431-54043-4
912 _aZDB-2-CMS
999 _c104035
_d104035